China's First Exploration of Chukchi Sea and Its Adjacent Waters in the Arctic -A Study on Lead Geochemistry of Atmospheric Aerosol

(整期优先)网络出版时间:2003-01-11
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ThePbconcentrationsofatmosphericaerosolintheChukchiSeaoftheArcticvarywithintherangeof0.167-0.962ng/m3,withanaverageof0.532ng/m3.Theseconcentra-tionvaluesare200timeshigherthanthenaturalbackgroundvaluesofsnowsamplesthere.Cal-culationofthePbenrichmentfactorofaerosolindicatesthattheocean-andcontinent-sourceleadaccountfor9.23%and0.01%,respectively,butindustriallyreleasedPbaccountsformorethan90%oftheatmosphericPb.ThePbisotopiccompositionofaerosolhasrevealedthatthesourcesofleadfromindustrialleadthatcausespollutionincludemainlythewesternpartofNorthAmerica,EastEuropeandtheformerSovietUnion.ThecalculationofthetotalfalloutfluxofPbindicatesthatthemeanvalueofinputfluxintotheChukchiSeais0.02mgm-2a-1,equivalenttothatofsouthernPacificbutslightlylowerthanthatofnorthernIndianSeaandsouthernAtlantic.ItisevidencedthatthePbinputfluxintotheChukchiSeaisfarlowerthanthatofftheBalticSea,theNorthSeaandtheMediterraneanSea.