简介：Magnetoplasmonicsensorsareattractivecandidatesforultrasensitivechemicalandbiomedicalsensorapplications.Avarietyofferromagneticmetalthinfilmshavebeenusedformagnetoplasmonicdeviceapplications,yetthedependenceofsensorperformanceontheopticalandmagneto-opticalpropertiesofferromagneticmetalmaterialshasbeenrarelystudied.Inthiswork,wereportthestudyofenhancedmagneto-opticalKerreffect（MOKE）andsensingperformanceinAu∕FexCo1-xbilayermagneto-opticalsurfaceplasmonresonance（MOSPR）transducers.TheopticalconstantsofFexCo1-x（x=0,0.29,0.47,0.65,and1）inasputter-depositedAu∕FexCo1-xdevicearecharacterizedbytheattenuatedtotalinternalreflection（ATR）method.FexCo1-xthinfilmsshowdifferentMOKEsasafunctionofthechemicalconcentration,withthehighesttransverseMOKEsignalobservedinFe0.7Co0.3.Indexsensingperformanceiscloselyrelatedtothematerial’sopticalandmagneto-opticalconstants.BystudyingthesensingperformanceintheparameterspaceoftheAu∕FexCo1-xbilayerthicknesses,thehighestsensitivityisfoundtobe0.385（theoretical）and0.306RIU-1（experimental）intheAu∕Fe0.7Co0.3MOSPRdevices.OurresearchhighlightstheinfluenceoftheopticalpropertiesofferromagneticmaterialtodevicesensitivityinMOSPRtransducers.ThehighsensitivityinAu∕FexCo1-xMOSPRdevicesmakethesestructuresattractivecandidatesforchemicalandbiomedicalsensingapplications.

简介：我们在Mn50Ni40SnSbx(x=1，2，3，和4)合金。所有准备样品在房间温度与空间组一起展出B2类型结构。Sb的替换增加原子价电子集中并且减少联合起来的房间体积。作为结果，当x增加，magnetostructural转变向更高的温度很快变。在在不同磁场变化下面的磁性的熵的变化在这转变附近被探索。等温的磁化曲线展出典型metamagnetic行为，显示magnetostructural转变能被一个磁场导致。悦耳的martensitic转变和磁性的熵变化建议那Mn50Ni40SnSbx合金是应用在的吸引人的候选人固态制冷。

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简介：ThispaperprovidesareviewonsampleinjectorswhichareprovidedatSPring-8AngstromCompactfreeelectronLAser(SACLA)forconductingserialmeasurementina‘diffract-before-destroy'schemeusinganx-rayfreeelectronlaser(XFEL).VersatileexperimentalplatformsatSACLAareabletoacceptvarioustypesofinjectors,amongwhichliquidjet,dropletandviscouscarrierinjectorsarefrequentlyutilized.Theseinjectorsproducedifferentformsoffluidtargetssuchasaliquidfilamentwithadiameterintheorderofmicrometer,micro-dropletsynchronizedtoXFELpulses,andslowlyflowingcolumnofhighlyviscousfluidwitharatebelow1μLmin-1.Characteristicsandapplicationsoftheinjectorsaredescribed.

简介：分析了X射线辐照电缆的物理过程,建立了基于有限元方法的二维诺顿等效电流源计算模型,将泊松方程、电场强度、电荷守恒方程等求解过程转换为矩阵和向量运算,并利用PETSc程序包编程计算,模拟了辐射感应电导率和间隙效应对屏蔽电缆X射线辐照响应的影响。结果显示,仅考虑辐射感应电导率效应时,随着X射线注量的增加,诺顿等效电流源逐渐趋于饱和,波形宽度变窄,并逐渐变为双极性波形。仅考虑间隙效应时,诺顿等效电流源幅度与间隙宽度近似成正比;间隙效应会大幅抵消辐射感应电导率效应的影响,诺顿等效电流源幅度仍近似正比于间隙宽度。该方法实现了电缆X射线辐照非线性效应的模拟,并将计算对象扩展到屏蔽多导体电缆。

简介：TheadsorptionofCOonPtgroupmetals,asamostfundamentalelementaryreactionstep,hasbeenwidelystudiedincatalysisandelectrocatalysis.Particularly,thestructuresofCOonPt(111)havebeenextensivelyinvestigated,owingtoitsimportancetobothfundamentalandappliedcatalysis.Yet,muchlessisknownregardingCOadsorptiononaPt(111)surfacemodulatedbysupportedoxidenanostructures,whichisofmorerelevancetotechnicalcatalysis.Wethusinvestigatedthecoverage-dependentadsorptionofCOonaPt(111)surfacepartiallycoveredbyFeOxnanostructures,whichhasbeendemonstratedasaremarkablecatalystforlow-temperatureCOoxidation.Wefoundthat,duetoitsstrongchemisorption,thecoverage-dependentstructureofCOonbarePtisnotinfluencedbythepresenceofFeOx.But,oxygen-terminatedFeOxnanostructurescouldmodulatethediffusivityofCOattheirvicinity,andthusaffecttheformationoforderedCOsuperstructuresatlowtemperatures.Usingscanningtunnelingmicroscopy(STM),weinspectedthediffusivityofCO,followedthephasetransitionsofCOdomains,andresolvedthemoleculardetailsofthecoverage-dependentCOstructures.OurresultsprovideafullpictureforCOadsorptiononaPt(111)surfacemodulatedbyoxidenanostructuresandshedlightsontheinter-adsorbateinteractiononmetalsurfaces.

简介：WeinvestigatethesensitivityoftheangularrotationmeasurementwiththemethodofhomodynedetectioninSU（2）andSU（1,1）interferometersbyemployingorbitalangularmomentum（OAM）.BycombiningacoherentbeamwithavacuumbeaminanSU（2）interferometer,wegetthesensitivityoftheangularrotationmeasurementas1/(2N1/2l).WecansurpassthelimitoftheangularrotationmeasurementinanSU（1,1）interferometerbycombiningacoherentbeamwithavacuumbeamorasqueezedvacuumbeamwhentheprobebeamhasOAM.Withoutinjection,thesensitivitycanreach1/(2N1/2l).Inaddition,byemployinganotherconstructionofanSU（1,1）interferometerwherethepumpbeamhasOAM,withthesameinjectionofanSU（1,1）interferometer,thesensitivityoftheangularrotationmeasurementcanbeimprovedbyafactorof2,reaching1/（4Nl）.Theresultsconfirmthepotentialofthistechnologyforprecisionmeasurementsinangularrotationmeasurements.

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简介：Thecomplexbandstructuresofa1Danisotropicgraphenephotoniccrystalareinvestigated,andthedispersionrelationsareconfirmedusingthetransfermatrixmethodandsimulationofcommercialsoftware.Itisfoundthattheresultofusingeffectivemediumtheorycanfitthederiveddispersioncurvesinthelowwavevector.Transmission,absorption,andreflectionatobliqueincidentanglesarestudiedforthestructure,respectively.Omni-gapsexistforanglesashighas80°fortwopolarizations.Physicalmechanismsofthetunabledispersionandtransmissionareexplainedbythepermittivityofgrapheneandtheeffectivepermittivityofthemultilayerstructure.

简介：TogaindeepinsightintotheMorphologicaleffectofNixMg1-xOcatalystsonthereactionofCO2reformingwithmethane,wedesignedandfabricatedthreedifferentspatialstructuralNixMg1-xOcatalysts.TheseNixMg1-xOcatalystswithspecificmodelssuchasrod,sheetandsphere,exhibitedvariousactivityandstabilityinCO2reformingreaction.HereinNixMg1-xOnanorodsdisplayedhighercatalyticactivity,inwhichmethaneconversionwasupto72%andCO2conversionwas64%at670°Cwithaspacevelocityof79,200mL/（gcath）,comparedwithnanosheetandnanospherecounterparts.Furthermore,bothcatalystsofNixMg1-xOnanorodandnanosheetshowedahighresistancetowardcokedepositionandsinteringofactivesitesintheprocessofCO2reformingofmethane.

简介：针对红外探测器在空间应用中受高能粒子辐照后性能衰退的问题,利用电子束辐照实验,开展了位移损伤对HgCdTe材料红外透射光谱影响的研究.通过对比辐照前后材料的性能变化,结合光在材料中的传播过程及半导体辐射效应理论,分析了位移损伤对HgCdTe材料红外透射光谱的影响机制.结果表明：HgCdTe材料经电子辐照后,红外透射光谱发生衰退,衰退的幅度随辐照注量的增大而增大,且短波方向上的衰退幅度大于长波方向上的衰退幅度.该工作可为深入开展HgCdTe红外探测器辐射损伤效应及损伤机理的研究提供参考.

简介：LiMn2O4andLiNixAlyMn2-x-yO4（x=0.50;y=0.05-0.50）powdershavebeensynthesizedviafacilesolgelmethodusingBehenicacidasactivecheiatingagent.Thesynthesizedsamplesaresubjectedtophysicalcharacterizationssuchasthermogravimetricanalysis（TG/DTA）,X-raydiffraction（XRD）,Fouriertransforminfraredspectroscopy（FT-IR）,field-emissionscanningelectronmicroscopy（FESEM）,transmissionelectronmicroscopy（TEM）andelectrochemicalstudiesviz.,galvanostaticcyclingproperties,electrochemicalimpedancespectroscopy（EIS）anddifferentialcapacitycurves（dQ/dE）.FingerprintXRDpatternsofLiMn2O4andLiNixAlyMn2-x-yO4fortifythehighdegreeofcrystallinitywithbetterphasepurity.FESEMimagesoftheundopedpristinespinelillustrateuniformsphericalgrainssurfacemorphologywithanaverageparticlesizeof0.5μmwhileNidopedparticlesdepictthesphericalgrainsgrowth（50nm）withice-cubesurfacemorphology.TEMimagesofthespinelLiMn2O4showstheuniformsphericalmorphologywithparticlesizeof（100nm）whilelowlevelofAl-dopingspinel（LiNio.5Alo.05Mn1.45O4）displayingcloudyparticleswithagglomeratedparticlesof（50nm）.TheLiMn2O4samplescalcinedat850℃deliverthedischargecapacityof130mAh/ginthefirstcyclecorrespondsto94%coiumbicefficiencywithcapacityfadeof1.5mAh/g/cycleovertheinvestigated10cycles.Amongallfourdopantcompositionsinvestigated,LiNi0.5Al0.05Mn1.45O4deliversthemaximumdischargecapacityof126mAh/gduringthefirstcycleandshowsthestablecyclingperformancewithlowcapacityfadeof1mAh/g/cycle（capacityretentionof92%）overtheinvestigated10cycles.ElectrochemicalimpedancestudiesofspinelLiMn2O4andLiNi0.5Al0.05Mn1.45O4depictthehighandlowrealpolarizationof1562and1100Ω.

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简介：Atheoreticaldesignispresentedfora1×Mwavelength-selectiveswitch（WSS）thatroutesanyoneofNincomingwavelengthsignalstoanyoneofMoutputports.Thisplanaron-chipdevicecomprisesofa1×Ndemultiplexer,agroupofNswitching'trees'actuatedbyelectro-opticalorthermo-opticalmeans,andanM-foldsetofN×1multiplexers.Treesutilize1×2switches.TheWSSinsertionlossisproportionalto(log2（M+N+1）)Alongwithcrosstalkfromtrees,crosstalkispresentateachcross-illuminatedwaveguideintersectionwithintheWSS,andthereareatmostN-1suchcrossingsperpath.TheselossandcrosstalkpropertieswilllikelyplaceapracticallimitofN=M=16upontheWSSsize.Byconstrainingthe1×2switchingenergyto1fJ∕bit,wefindthatresonant,narrowband1×2switchesarerequired.The1×2devicesproposedherearenanobeamMach–Zehndersandasymmetriccontra-directionalcouplerswithgratingassistance.

简介：为研究空间用四结太阳电池中InGaAsP/InGaAs子电池在电子辐照条件下的性能衰退情况,对InGaAsP/InGaAs双结电池开展了1MeV电子辐照试验,测试了辐照前后的电学参数和量子效率,分析讨论了参数退化情况.结果表明：随着电子注量和位移损伤剂量的增加,电池性能参数退化程度逐渐加大;由位移损伤缺陷导致的载流子寿命减小,是导致电池短路电流和开路电压下降的主要原因;InGaAsP/InGaAs双结电池基区损伤比发射区损伤更加严重,因此,提高其抗辐射能力的关键在于优化基区结构.

简介：Ceria-zirconiasolidsolutionhasbeenpreparedbytheureagrindcombustionandcitricacidsol-gelmethodsforcatalyticapplicationsasoxygenstorage/releasematerialsinthisstudy.Thepropertiesandoxygenstorage/releasecapacitiesofsampleswithdifferentZrcontentswerecharacterizedandevaluatedbyX-raydiffraction（XRD）,N2adsorption,scanningelectronmicroscopy（SEM）,Ramanspectroscopy,andinsituCO–CO2loopingtest.Theresultsdemonstratethatthesamplespreparedbytwomethodsareallofexcellentlattice[O]release/storagepropertiesandmaintaingoodlong-termcyclestability.ButthepreparationmethodsignificantlyimpactsthehomogeneityofsamplesrelatedtotheirredoxpropertiesandthecontentofZrover20%,whichgreatlychangedthepropertiesofceria-zirconiasolidsolutionsandcausedtheirchangingofcrystallinesymmetryfromcubictotetragonal.Thesamplespreparedbycitricacidsolgelmethodareofmorehomogeneousparticlesizesandhigherspecificsurfaceareasthanthatbyureagrindcombustionmethod,whichisbenefittotheoxygenreleaseratherthanoxygenstorage.ThebulkoxygenamountmigratedtosurfaceincreaseswiththeincreasingZrcontent,however,theamountoflatticeoxygenmigrationdecreaseswhenZrcontentisover20%.WhenZrcontentis20%,thedifferencesofstorage/releasecapacitiesfromtwodifferentpreparationmethodsarereducedathightemperatureinthelong-termloopreaction.

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